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Two new μ4-O bridged hexanuclear lanthanide complexes, [Dy6L′4(μ4-O)(NO3)4]·4CH3OH (1) and [Sm6L′4(μ4-O)(CH3COO)4]·2CH3OH (2), have been assembled by using methyl modified Schiff-base ligand H3L′ (2,6-bis((2-hydroxypropylimino)methyl)-4-methylphenol). The complex 1 shares a similar μ4-O bridged Dy6 core as the parent Dy6-2, while coordination geometries and magnetic interactions are slightly changed upon the modulation of the ligand, which results in distinct single-molecule magnetic (SMM) and single-molecule toroic (SMT) properties.

The effect of additional methyl on the magnetic relaxation and toroidal moment of Dy6 complex

The effect of additional methyl on the magnetic relaxation and toroidal moment of Dy₆ complex