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Four organic sensitizers having a di-branched molecular structure D–(π–A)2 (D = para-substituted arylamine, π = 9,9-dibutylfluorene, A = cyanoacrylic acid) were synthesized, characterized, and applied in the development of dye-sensitized solar cells (DSSCs). It was found that the nature of the para-substituent affects the behavior of these sensitizers. In particular, the introduction of a C11 linear fluorous alkoxy group led to an improvement in the power conversion efficiency with respect to the commonly employed nonfluorous alkoxy substituents.

new journal of chemistry

Fluorous molecules for dye-sensitized solar cells: synthesis and properties of di-branched, di-anchoring organic sensitizers containing fluorene subunits