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The unsymmetric P III /P V cyclodiphosphazane framework [(S[double bond, length as m-dash])(H)P(μ-N  Bu) 2 PNH  Bu] (2) provides entry into the mixed chalgogenide dianion [(S)P(μ-N  Bu) 2 P(Se)N  Bu] 2- , and unique insight into the mechanisms of cis/trans isomerism in phosph(iii)- and phosph(v)-azanes.

Isomerisation, reactivity and coordination chemistry of a new hybrid, multi-functional phosphazane