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A coordination complex containing thioindigo (TI 2− ) dianions and Cr 3+ with a high S = 3/2 spin state and salt {cryptand[2,2,2](Na + )}(TI˙ − ) ( 2 ) with paramagnetic TI˙ − radical anions have been studied for the first time.

dalton transactions

cis-Thioindigo (TI) – a new ligand with accessible radical anion and dianion states. Strong magnetic coupling in the {[TI-(μ<sub>2</sub>-O),(μ-O)]Cp*Cr}<sub>2</sub>dimers

cis-Thioindigo (TI) – a new ligand with accessible radical anion and dianion states. Strong magnetic coupling in the {[TI-(μ2-O),(μ-O)]Cp*Cr}2dimers

cis-Thioindigo (TI) – a new ligand with accessible radical anion and dianion states. Strong magnetic coupling in the {[TI-(μ₂-O),(μ-O)]Cp*Cr}₂dimers