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1 and 2 were synthesized through the complexation of 5,10,15,20-tetra-4-pyridyl-21H,23H-porphine with copper(II) acetate and copper(II) 1-naphthoate and exhibited two-dimensional open and closed form structures, respectively. X-ray diffraction identified the supramolecular interactions leading to these packing motifs. N2 and CO2 sorption isotherms indicate that 2 allows the separation of these gases.

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Supramolecular porphyrin-based metal–organic frameworks: Cu(<scp>ii</scp>) naphthoate–Cu(<scp>ii</scp>) tetrapyridyl porphine structures exhibiting selective CO<sub>2</sub>/N<sub>2</sub> separation

Supramolecular porphyrin-based metal–organic frameworks: Cu(ii) naphthoate–Cu(ii) tetrapyridyl porphine structures exhibiting selective CO2/N2 separation

Supramolecular porphyrin-based metal–organic frameworks: Cu(ii) naphthoate–Cu(ii) tetrapyridyl porphine structures exhibiting selective CO₂/N₂ separation