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In aqueous solution, host-guest complexation is frequently driven by the hydrophobic effect, which also constitutes a popular approach in the design of supramolecular assemblies. Herein, we report an orthogonal assembly motif, the chaotropic effect, which exploits the tendency of chaotropic anions to associate with hydrophobic surfaces.

The chaotropic effect as an orthogonal assembly motif for multi-responsive dodecaborate-cucurbituril supramolecular networks