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Electrochemical reduction of an azoniahelicene affords a dimer, accompanied by a strong change in the electronic circular dichroism. The fast dimerisation event leads to a &gt;500 mV shift of the oxidation potential, affording a large area of bistability, where the chiroptical signal only depends on the redox history.

Intense redox-driven chiroptical switching with a 580 mV hysteresis actuated through reversible dimerization of an azoniahelicene