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Two M 8 L 12 cubic coordination cages, as desolvated crystalline powders, preferentially adsorb CO 2 over N 2 with ideal selectivity CO 2 /N 2 constants of 49 and 30 at 298 K. A binding site for CO 2 is suggested by crystallographic location of CS 2 within the cage cavity at an electropositive hydrogen-bond donor site, potentially explaining the high CO 2 /N 2 selectivity compared to other materials with this level of porosity.

Highly selective CO2vs. N2 adsorption in the cavity of a molecular coordination cage

Highly selective CO₂vs. N₂ adsorption in the cavity of a molecular coordination cage