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The photocatalytic production of hydrogen peroxide from water and dioxygen under visible light irradiation was made possible by using polymeric cyano-bridged heteronuclear metal complexes (M II [Ru II (CN) 4 (bpy)]; M II = Ni II , Fe II and Mn II ), where the photocatalytic two-electron reduction of O 2 and water oxidation were catalysed by the Ru and M II moieties, respectively.

chemical communications

Dual function photocatalysis of cyano-bridged heteronuclear metal complexes for water oxidation and two-electron reduction of dioxygen to produce hydrogen peroxide as a solar fuel