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Nano-assembled capsules can incorporate large payloads of high relaxivity Gd 3+ , permitting the development of highly detectable molecular imaging agents for MRI. A new encapsulating shell, based upon cross-linked peptides, is found to afford smaller capsules (127 nm average diameter) with exceptionally high per-Gd 3+ relaxivities (70.7 s -1 mmolal -1 ).

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Crosslinked shells for nano-assembled capsules: a new encapsulation method for smaller Gd<sup>3+</sup>-loaded capsules with exceedingly high relaxivities

Crosslinked shells for nano-assembled capsules: a new encapsulation method for smaller Gd3+-loaded capsules with exceedingly high relaxivities

Crosslinked shells for nano-assembled capsules: a new encapsulation method for smaller Gd³⁺-loaded capsules with exceedingly high relaxivities