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Successful nanostructuration approaches developed in the last few years have allowed the preparation of robust valence tautomeric (VT) switchable (micro-/nano-) structures of a variety of dimensions and morphologies. These results are expected to definitely foster the implementation of these materials on hybrid molecular electronic devices but also endorse new applications in other different fields such as sensing, drug delivery or water remediation, among others.N. A. V.-M. thanks the Ministerio de Ciencia e Innovación (MICINN) for a predoctoral FPU fellowship. M. G. thanks the CSIC for a predoctoral grant (JAEpre). C. B. thanks the ICN2 and the Severo Ochoa program for his predoctoral grant. This work was supported by projects MAT2015-70615-R and CTQ2015-65439-R from the Spanish Government and by FEDER funds. ICN2 acknowledges support from the Severo Ochoa Program (MINECO, Grant SEV-2013-0295).We acknowledge support by the CSIC Open Access Publication Initiative through its Unit of Information Resources for Research (URICI).Peer Reviewe

journal of materials chemistry. c

Switchable colloids, thin-films and interphases based on metal complexes with non-innocent ligands: the case of valence tautomerism and their applications