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It is highly desirable but challenging to develop bifunctional electrocatalysts for efficiently boosting both the oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) in energy storage and conversion devices. Here, a simple yet cost-efficient thermal annealing strategy is developed to synthesize FeP embedded in N, P dual-doped 2D porous carbon nanosheets (FeP@NPCs). The obtained FeP@NPCs exhibited outstanding catalytic activities and durabilities toward both the ORR and OER with a potential gap of 0.74 V between the half-wave potential for the ORR and the OER potential at a current density of 10 mA cm−2 in alkaline electrolytes.

FeP embedded in N, P dual-doped porous carbon nanosheets: an efficient and durable bifunctional catalyst for oxygen reduction and evolution reactions