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Highly dispersible TiO2@ZrO2 nanoparticles are synthesized to prepare an ultra-flat and crack-free spacer film, leading to an enhanced insulating ability compared to a conventional spacer. The average power conversion efficiency of fully printable mesoscopic perovskite solar cells is improved from 10.2% to 12.5%, and the highest steady output power conversion efficiency is 13.8%.

Spacer improvement for efficient and fully printable mesoscopic perovskite solar cells