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Despite recent advances in main group N-heterocyclic carbene (NHC) coordination chemistry, gallium hydrides remain, in large part, an unexplored area of research. In this paper we outline efficient routes to azide- and amido-functionalized gallium hydrides such as NHC·GaH 2 N 3 and NHC·GaH 2 N(SiMe 3 ) 2 and explore these species as potential precursors to HGaNH complexes and bulk gallium nitride (GaN).

Azido- and amido-substituted gallium hydrides supported by N-heterocyclic carbenes