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Manganese dioxide nanosheet arrays with interconnected arrangements are easily synthesized on vapor grown carbon fibers (MnO 2 NSAs@VCFs) by a simple wet-chemical method at low temperature. The conductive nature of the VCFs serves as a scaffold and easily reduces potassium permanganate species for the formation of hierarchical MnO 2 NSAs@VCFs. When utilized as an electroactive material for pseudocapacitors, the sophisticated configuration of the nanocomposite provides an effective electrochemical activity and an electron pathway for higher electrochemical performance in 1 M Na 2 SO 4 aqueous solution. The hierarchical MnO 2 NSAs@VCFs exhibit a maximum specific capacitance of 115.3 F g -1 at a current density of 0.5 A g -1 with an excellent cycling stability of 85.6% after 2000 cycles at a current density of 5 A g -1 . Such facile and cost-effective fabrication of a metal oxide nanocomposite with improved electrochemical performance allows it to be considered as a promising electroactive material for energy storage devices.

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Birnessite-type MnO<sub>2</sub> nanosheet arrays with interwoven arrangements on vapor grown carbon fibers as hybrid nanocomposites for pseudocapacitors

Birnessite-type MnO2 nanosheet arrays with interwoven arrangements on vapor grown carbon fibers as hybrid nanocomposites for pseudocapacitors

Birnessite-type MnO₂ nanosheet arrays with interwoven arrangements on vapor grown carbon fibers as hybrid nanocomposites for pseudocapacitors