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Interpretation of catalytic performance during the MTH process is hampered by heat transport phenomena. We demonstrate that large temperature rises can occur during fixed bed labscale catalyst testing of ZSM-5, even when a large catalyst bed dilution is applied. Formation of mesopores in ZSM-5 leads to partial mitigation of these effects because of a lower generation of heat per unit catalyst volume and weakening of the zeolite acidity

The importance of heat effects in the methanol to hydrocarbons reaction over ZSM-5: on the role of mesoporosity on catalyst performance