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Perovskite solar cells (PSC) are shown to behave as coupled ionic-electronicconductors with strong evidence that the ionic environment moderates both therate of electron-hole recombination and the band offsets in planar PSC.Numerous models have been presented to explain the behavior of perovskite solarcells, but to date no single model has emerged that can explain both thefrequency and time dependent response of the devices. Here we present astraightforward coupled ionic-electronic model that can be used to explain thelarge amplitude transient behavior and the impedance response of PSC.

Microseconds, milliseconds and seconds: deconvoluting the dynamic behaviour of planar perovskite solar cells