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This work investigates the production of molecular hydrogen isotopologues (H 2 , HD, and D 2 ) during low energy electron irradiation of layered and isotopically labelled thin films of amorphous solid water (ASW) in ultrahigh vacuum. Experimentally, the production of these molecules with both irradiation time and incident electron energy in the range 400 to 500 eV is reported as a function of the depth of a buried D 2 O layer in an H 2 O film. H 2 is produced consistently in all measurements, reflecting the H 2 O component of the film, though it does exhibit a modest reduction in intensity at the time corresponding to product escape from the buried D 2 O layer. In contrast, HD and D 2 production exhibit peaks at times corresponding to product escape from the buried D 2 O layer in the composite film. These features broaden the deeper the HD or D 2 is formed due to diffusion. A simple random-walk model is presented that can qualitatively explain the appearance profile of these peaks as a function of the incident electron penetration.

Molecular hydrogen production from amorphous solid water during low energy electron irradiation