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Graphitic carbon nitride (g-C 3 N 4 ) synthesised from a urea precursor is an excellent CO 2 reduction photocatalyst using [Co(bpy) n ] 2+ as a co-catalyst. A five-fold increase in activity for the highly polymerised urea derived g-C 3 N 4 is achieved compared to alternative precursors. Transient absorption, time-resolved and steady-state emission studies indicate that the enhanced activity is related to both an increased driving force for photoelectron transfer and a greater availability of photogenerated charges.

Photochemical CO2 reduction using structurally controlled g-C3N4

Photochemical CO₂ reduction using structurally controlled g-C₃N₄