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A hydrogen bond-driven supramolecular strategy to synthesize multiphase-Fe anchoring on hierarchical N-doped graphitic carbon was proposed. As a result, the as-obtained catalysts showed unusual trifunctional activities in the oxygen reduction reaction, oxygen evolution reaction and hydrogen evolution reaction, even surpassing noble-metal catalysts such as Pt/C and RuO 2 .

Coupling multiphase-Fe and hierarchical N-doped graphitic carbon as trifunctional electrocatalysts by supramolecular preorganization of precursors