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A β-SiH functionalized benzyl anion [C(SiHMe 2 ) 2 Ph] - is obtained by deprotonation of HC(SiHMe 2 ) 2 Ph with KCH 2 Ph or by reaction of KOtBu and (Me 2 HSi) 3 CPh; LnI 3 (THF) n and three equivalents of this carbanion combine to provide homoleptic tris(alkyl)lanthanide compounds Ln{C(SiHMe 2 ) 2 Ph} 3 (Ln = La, Ce, Pr, Nd) containing secondary metal-ligand interactions.

Homoleptic organolanthanide compounds supported by the bis(dimethylsilyl)benzyl ligand