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Hydrogen release from Al-based complex hydrides composed of metal cation(s) and [AlH 4 ] - was investigated using inelastic neutron scattering viewed from vibrational dynamics. The hydrogen release followed the softening of translational and [AlH 4 ] - librational modes, which was enhanced by vibrational dynamics and the valence(s) of the metal cation(s).

Hydrogen release reactions of Al-based complex hydrides enhanced by vibrational dynamics and valences of metal cations