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We demonstrate, for the first time, that a hydrogen-bonded low-density organic framework can be applied as a platform to achieve periodic alignment of paired molecules of C60, which is the smallest example of a finite-numbered cluster of C60. The framework is a layered assembly of a hydrogen-bonded 2D hexagonal network (LA-H-HexNet) composed of dodecadehydrotribenzo[18]annulene derivatives.

Alignment of paired molecules of C60 within a hexagonal platform networked through hydrogen-bonds

Alignment of paired molecules of C₆₀ within a hexagonal platform networked through hydrogen-bonds