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We report the direct splitting of pure water by light-excited graphitic carbon nitride (g-C 3 N 4 ) modified with Pt, PtO  x  , and CoO  x  as redox cocatalysts, while pure g-C 3 N 4 is virtually inactive for overall water splitting by photocatalysis. The novelty is in the selective creation of both H 2 and O 2 cocatalysts on surface active sites of g-C 3 N 4  via photodeposition triggering the splitting of water for the simultaneous evolution of H 2 and O 2 gases in a stoichiometric ratio of 2 : 1, irradiated with light, without using any sacrificial reagents. The photocatalyst was stable for 510 hours of reaction.

Overall water splitting by Pt/g-C3N4photocatalysts without using sacrificial agents

Overall water splitting by Pt/g-C₃N₄photocatalysts without using sacrificial agents