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We discovered an extremely suitable sacrificial electron donor, 1,3-dimethyl-2-( o -hydroxyphenyl)-2,3-dihydro-1 H -benzo[ d ]imidazole, for the selective photocatalytic reduction of CO 2 to formic acid using a Ru(ii)-Ru(ii) supramolecular photocatalyst. The efficiency, durability, and rate of photocatalysis are significantly increased ( Φ  HCOOH = 0.46, TON HCOOH = 2766, TOF HCOOH = 44.9 min -1 ) in comparison with those using 1,3-dimethyl-2-phenyl-2,3-dihydro-1 H -benzo[ d ]imidazole or 1-benzyl-1,4-dihydronicotinamide.

Highly efficient, selective, and durable photocatalytic system for CO2 reduction to formic acid

Highly efficient, selective, and durable photocatalytic system for CO₂ reduction to formic acid