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Preparation of well-interconnected TiO2 electrodes at low temperature is critical for the fabrication of\udhighly efficient dye-sensitized solar cells (DSCs) on plastic substrates. Herein we explore a synergistic\udapproach using a combination of chemical and physical sintering. We formulate a binder-free TiO2 paste\udbased on “nanoglue” as the chemical sintering agent, and use it to construct a photoelectrode on plastic\udby low-temperature physical compression to further improve the connectivity of TiO2 films. We\udsystematically investigated the factors affecting the photovoltaic performance and found the conditions\udto achieve electron diffusion lengths as long as 25 mm and charge collection efficiencies as high as 95%,\udas electrochemical impedance spectroscopy measurements indicate. We apply this approach to obtain a\udDSC deposited on plastic displaying 6.4% power conversion efficiency based on commercial P25 titania\udparticlesPeer reviewe

rsc advances

Synergistic strategies for the preparation of highly efficient dye-sensitized solar cells on plastic substrates: combination of chemical and physical sintering