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[(Li0.8Fe0.2)OH]FeS and the series [(Li0.8Fe0.2)OH]Fe(S1-xSex) (0<x<1) weresynthesized by hydrothermal methods and characterized by X-ray single crystaland powder diffraction, EDX and chemical analysis. Selenium-rich compounds showthe coexistence of magnetic ordering with superconductivity known from the pureselenium compound. Sulphur doping decreases the critical temperature throughchemical pressure until superconductivity is completely absent in[(Li0.8Fe0.2)OH]FeS, while the ferromagnetism in the [(Li0.8Fe0.2)OH] layerspersists. The Li:Fe ratio in the hydroxide layer, and thus the charge transferof 0.2 electrons from the hydroxide to the iron chalcogenide layers remainsunchanged in [(Li0.8Fe0.2)OH]Fe(S1-xSex), which indicates that the chemicalpressure effect of the smaller sulphide ions impedes superconductivity in[(Li0.8Fe0.2)OH]FeS

[(Li0.8Fe0.2)OH]FeS and the ferromagnetic superconductors [(Li0.8Fe0.2)OH]Fe(S1-xSex) (0