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In this work, the design, synthesis, and characterization of a donor–acceptor polymer from dithieno[3,2-b:2′,3′-d]pyrrole and isoindigo (i-ID) are presented. The synthesized polymer has been applied in the fabrication of large area ITO-free organic photovoltaic devices, both by spin coating and roll coating; the latter was used to construct both single junction and multi-junction organic photovoltaic (OPV) architectures.

journal of materials chemistry. c

An isoindigo containing donor–acceptor polymer: synthesis and photovoltaic properties of all-solution-processed ITO- and vacuum-free large area roll-coated single junction and tandem solar cells