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We report the first example of the use of enzymes to trigger the self-assembly of the conjugates of nucleobases, amino acids, and saccharide to form supramolecular hydrogels in water, which illustrates a facile approach for the development of a new class of multifunctional soft materials for biomedical applications.

Enzyme-instructed self-assembly of hydrogelators consisting of nucleobases, amino acids, and saccharide