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Epitaxial films of Li2MnO3 were synthesized using pulsed laser deposition. A 12.6 nm film exhibited a high discharge capacity of over 300 mA h g(-1) following its fiftieth cycle and better stability than 29.8 and 47.8 nm films. The surfaces of such films are intrinsically active at the electrochemical interface.

Highly reversible capacity at the surface of a lithium-rich manganese oxide: a model study using an epitaxial film system