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A highly stereoselective one-pot procedure involving an enantioselective Michael addition promoted by low loading of an amino-squaramide catalyst followed by an achiral base catalyzed domino Michael-Knoevenagel-type 1,2-addition sequence provides efficient access to fully substituted cyclohexanes bearing five contiguous stereogenic centers in good yields (68-86%) and excellent stereoselectivities (&gt;30 : 1 dr and 96-99% ee).

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Asymmetric synthesis of functionalized cyclohexanes bearing five stereocenters<i>via</i>a one-pot organocatalytic Michael–Michael–1,2-addition sequence

Asymmetric synthesis of functionalized cyclohexanes bearing five stereocentersviaa one-pot organocatalytic Michael–Michael–1,2-addition sequence