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trans-[OsVI(tmc)(O)2]2+ (tmc = 1,4,8,11-tetramethyl-1,4,8,11-tetra-azacyclotetradecane) and trans-[Os VI(CN)4(O)2]2- are emissive in the solid state and in fluid solutions at room temperature (τ ∼ 1.0-1.5 μs); the 3Eg state of trans-[OsVI(tmc)(O) 2]2+ is a powerful one-electron oxidant {[Os VI(O)2]2+ + e- → [Os V(O)2]+, Ef 0 > 2.0 V vs. normal hydrogen electrode} in aqueous solution, reacting with PPh 3 and (PhCH2)2S to give O=PPh3 and (PhCH2)2S=O, respectively.link_to_subscribed_fulltex

journal of the chemical society chemical communications

Metal–oxo photo-oxidants. Photochemistry and photophysics of trans-[OsVI(tmc)(O)2]2+(tmc = 1,4,8,11-tetramethyl-1,4,8,11-tetra-azacyclotetradecane) and trans-[OsVI(CN)4(O)2]2–