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4-Methylpyrimidine-2-thione reacts with methylmercury hydroxide to give the thiolate derivative HgMe(SC4H2N2Me-2), the X-ray structure of which reveals pairs of molecules with a mercury–mercury distance of 3.10 A.

Methyl(2-mercapto-4-methylpyrimidinato)mercury(II): a methylmercury(II) derivative with an unusual metal–metal interaction