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A metal-organic framework (MOF), NH(2)-MIL-101(Al), which acts as a bifunctional, site-isolated Lewis acid-Brønsted base heterogeneous catalyst, catalyzes a tandem Meinwald rearrangement-Knoevenagel condensation reaction with remarkable substrate selectivity.

Tandem catalysis with a bifunctional site-isolated Lewis acid–Brønsted base metal–organic framework, NH2-MIL-101(Al)