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We report here on one of the rare cases that realizes a reductive charge shift from a primary electron acceptor (C60) to a secondary electron acceptor (C70) in a ZnP–C60–C70 conjugate. Initially, charge separation evolves from an excited state electron donor (ZnP). By far the most far reaching benefit from such a reductive pathway is a marked slow down of the energy wasting charge recombination when compared to the ZnP–C60 conjugate (i.e., picoseconds versus nanoseconds).

Powering reductive charge shift reactions—linking fullerenes of different electron acceptor strength to secure an energy gradient