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In this paper we report the successful incorporation of phosphate and sulfate groups into the ionic conductor, Ba2In2O 5, with the samples analysed through a combination of X-ray diffraction, NMR, TGA, Raman spectroscopy and conductivity measurements. The results show that such oxyanion incorporation leads to a conversion from an ordered brownmillerite-type structure to a disordered perovskite-type, and hence increases the conductivity at temperatures <800 °C. In wet atmospheres, there is evidence for a significant enhancement of the conductivity through a protonic contribution.We would like to express thanks to the University of Birmingham for funding (EPS international studentship for JFS).Peer Reviewe

Oxyanion doping strategies to enhance the ionic conductivity in Ba2In2O5

Oxyanion doping strategies to enhance the ionic conductivity in Ba₂In₂O₅