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The comparison of the proportions of the minor products formed during the hydroisomerisation of n-butane over reduced MoO3 with thermodynamic data demonstrates that a bifunctional mechanism operates and that the rate-determining step is the isomerisation of the linear butene intermediates to iso-butene.

chemical communications

New insights into the reaction mechanism and the rate-determining step of n-butane hydroisomerisation over reduced MoO3 catalystsElectronic supplementary information (ESI) available: experimental details. See http://www.rsc.org/suppdata/cc/b3/b304978g/