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The combination of sensitive calorimetry, incoherent elastic neutron scattering and neutron di†raction hasbeen used to demonstrate the formation of solid layers containing both octane and nonane adsorbed ontographite from the binary alkane mixture. This combination of methods allow us to characterise the adsorbedlayer in some detail including the absolute composition and melting temperature as a function of solutioncomposition. The evidence presented here suggests that the two alkanes exist on the surface as patches of purematerial not as a single crystal incorporating both alkanes

The investigation of mixed monolayers adsorbed from solution: octane and nonane mixtures on graphite