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Pyridinol, a coordinating zwitter-ionic species serves as stoichiometrically loadable and non-leachable proton carrier. The partial replacement of the pyridinol by stronger hydrogen bonding, coordinating guest, ethylene glycol (EG), offers 1000-fold enhancement in conductivity (10 −6  to 10 −3  Scm −1 ) with record low activation energy (0.11 eV). Atomic modeling coupled with  13 C-SSNMR provides insights into the potential proton conduction pathway functionalized with post-synthetically anchored dynamic proton transporting EG moieties.

1000-fold enhancement in proton conductivity of a MOF using post-synthetically anchored proton transporters