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Experiment and theory evidence a new pathway for correlated two-electron release from many-body compounds following collective excitation by a single photon. Using nonequilibrium Green’s function approach we trace plasmon oscillations as the key ingredient of the effective electron-electron interaction that governs the correlated pair emission in a dynamic many-body environment. Results from a full  ab initio  implementation for C 60  fullerene are in line with experimental observations. The findings endorse the correlated two-electron photoemission as a powerful tool to access electronic correlation in complex systems.

Electron pair escape from fullerene cage via collective modes