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Recently monolayer jacutingaite (Pt 2 HgSe 3 ), a naturally occurring exfoliable mineral, discovered in Brazil in 2008, has been theoretically predicted as a candidate quantum spin Hall system with a 0.5 eV band gap, while the bulk form is one of only a few known dual-topological insulators that may host different surface states protected by symmetries. In this work, we systematically investigate both structure and electronic evolution of bulk Pt 2 HgSe 3  under high pressure up to 96 GPa. The nontrivial topology is theoretically stable, and persists up to the structural phase transition observed in the high-pressure regime. Interestingly, we found that this phase transition is accompanied by the appearance of superconductivity at around 55 GPa and the critical transition temperature  T  c  increases with applied pressure. Our results demonstrate that Pt 2 HgSe 3  with nontrivial topology of electronic states displays a ground state upon compression and raises potentials in application to the next-generation spintronic devices.

Pressure-induced superconductivity and structure phase transition in Pt2HgSe3