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Multiferroics and magnetoelectrics with coexisting and coupled multiple ferroic orders are materials promising new technological\udadvances. While most studies have focused on single-phase or heterostructures of inorganic materials, a new class of materials\udcalled metal–organic frameworks (MOFs) has been recently proposed as candidate materials demonstrating interesting new routes\udfor multiferroism and magnetoelectric coupling. Herein, we report on the origin of multiferroicity of (CH3)2NH2Mn(HCOO)3 via direct\udobservation of ferroelectric domains using second-harmonic generation techniques. For the first time, we observe how these\uddomains are organized (sized in micrometer range), and how they are mutually affected by applied electric and magnetic fields.\udCalculations provide an estimate of the electric polarization and give insights into its microscopic origin

Switchable electric polarization and ferroelectric domains in a metal-organic-framework