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We describe the first-principles design and subsequent synthesis of a newmaterial with the specific functionalities required for a solid-state-basedsearch for the permanent electric dipole moment of the electron. We showcomputationally that perovskite-structure europium barium titanate shouldexhibit the required large and pressure-dependent ferroelectric polarization,local magnetic moments, and absence of magnetic ordering even at liquid heliumtemperature. Subsequent synthesis and characterization ofEu$_{0.5}$Ba$_{0.5}$TiO$_3$ ceramics confirm the predicted desirableproperties.

First-principles design and subsequent synthesis of a material to search for the permanent electric dipole moment of the electron