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The hexahydro-1H-isoindolin-1-one core of muironolide A was prepared by asymmetric intramolecular Diels-Alder cycloaddition using a variant of the MacMillan organocatalyst which sets the C4,C5 and C11 stereocenters.

Assembly of the Isoindolinone Core of Muironolide A by Asymmetric Intramolecular Diels–Alder Cycloaddition