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Fluorescent defects in non-cytotoxic diamond nanoparticles are candidates forqubits in quantum computing, optical labels in biomedical imaging and sensorsin magnetometry. For each application these defects need to be optically andthermodynamically stable, and included in individual particles at suitableconcentrations (singly or in large numbers). In this letter, we combinesimulations, theory and experiment to provide the first comprehensive andgeneric prediction of the size, temperature and nitrogen-concentrationdependent stability of optically active NV defects in nanodiamonds.

Prediction and measurement of the size-dependent stability of fluorescence in diamond over the entire nanoscale