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Gold-molecule-gold junctions can be formed by carefully breaking a gold wirein a solution containing dithiolated molecules. Surprisingly, there is littleunderstanding on the mechanical details of the bridge formation process andspecifically on the role that the dithiol molecules play themselves. We proposethat alkanedithiol molecules have already formed bridges between the goldelectrodes before the atomic gold-gold junction is broken. This leads tostabilization of the single atomic gold junction, as observed experimentally.Our data can be understood within a simple spring model.

Stabilizing single atom contacts by molecular bridge formation