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We study interfacial water trapped between a sheet of graphene and amuscovite (mica) surface using Raman spectroscopy and ultra-high vacuumscanning tunneling microscopy (UHV-STM) at room temperature. We are able toimage the graphene-water interface with atomic resolution, revealing a layerednetwork of water trapped underneath the graphene. We identify water layernumbers with a carbon nanotube height reference. Under normal scanningconditions, the water structures remain stable. However, at greater electronenergies, we are able to locally manipulate the water using the STM tip.

Scanning Tunneling Microscopy Study and Nanomanipulation of Graphene-Coated Water on Mica