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A narrow Gaussian excluded volume potential, which tends to a delta-functionrepulsive potential in the limit of a width parameter d* going to zero, hasbeen used to examine the universal consequences of excluded volume interactionson the equilibrium and linear viscoelastic properties of dilute polymersolutions. Brownian dynamics simulations data, acquired for chains of finitelength, has been extrapolated to the limit of infinite chain length to obtainmodel independent predictions. The success of the method in predicting wellknown aspects of static solution properties suggests that it can be used as asystematic means by which the influence of solvent quality on both equilibriumand non-equilibrium properties can be studied.

macromolecules

Equilibrium Swelling and Universal Ratios in Dilute Polymer Solutions: <i>Exact</i> Brownian Dynamics Simulations for a Delta Function Excluded Volume Potential

Equilibrium Swelling and Universal Ratios in Dilute Polymer Solutions: Exact Brownian Dynamics Simulations for a Delta Function Excluded Volume Potential