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Conditions for the crossover from the strong to the superstrong segregation regime are analyzed for the case of comb−coil diblock copolymers. It is shown that the critical interaction energy between the components required to induce the crossover to the superstrong segregation regime is inversely proportional to mb = 1 + n/m, where n is the degree of polymerization of the side chain and m is the distance between successive grafting points. As a result, the superstrong segregation regime, being rather rare in the case of ordinary block copolymers, has a much better chance to be realized in the case of diblock copolymers with combs grafted to one of the blocks.

Domains in Melts of Comb−Coil Diblock Copolymers: Superstrong Segregation Regime