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We provide a simple and intuitive explanation for the interlayer slidingenergy landscape of metal dichalcogenides. Based on the recently introducedregistry index (RI) concept, we define a purely geometrical parameter whichquantifies the degree of interlayer commensurability in the layered phase ofmolybdenum disulphide (2HMoS2). A direct relation between the sliding energylandscape and the corresponding interlayer registry surface of 2H-MoS2 isdiscovered thus marking the registry index as a computationally efficient meansfor studying the tribology of complex nanoscale material interfaces in thewearless friction regime.

Interlayer Registry Determines the Sliding Potential of Layered Metal Dichalcogenides: The case of 2H-MoS2